Water-side turbulence enhancement of ozone deposition to the ocean

A parameterization for the deposition velocity of an ocean-reactive atmospheric gas (such as ozone) is developed. The parameterization is based on integration of the turbulent-molecular transport equation (with a chemical source term) in the ocean. It extends previous work that only considered reactions within the oceanic molecular sublayer. The sensitivity of the ocean-side transport to reaction rate and wind forcing is examined. A more complicated case with a much more reactive thin surfactant layer is also considered. The full atmosphere-ocean deposition velocity is obtained by matching boundary conditions at the interface. For an assumed ocean reaction rate of 103 s¿1, the enhancement for ozone deposition by oceanic turbulence is found to be up to a factor of three for meteorological data obtained in a recent cruise off the East Coast of the U.S.

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Main Authors: Fairall, C.W., Helmig, D., Ganzeveld, L.N., Hare, J.
Format: Article/Letter to editor biblioteca
Language:English
Subjects:boundary-layer, dry deposition, fluxes, gas-exchange, parameterization, surface, trends, wind-speed,
Online Access:https://research.wur.nl/en/publications/water-side-turbulence-enhancement-of-ozone-deposition-to-the-ocea
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spelling dig-wur-nl-wurpubs-3813992024-12-04 Fairall, C.W. Helmig, D. Ganzeveld, L.N. Hare, J. Article/Letter to editor Atmospheric Chemistry and Physics 2007 (2007) 7 ISSN: 1680-7316 Water-side turbulence enhancement of ozone deposition to the ocean 2007 A parameterization for the deposition velocity of an ocean-reactive atmospheric gas (such as ozone) is developed. The parameterization is based on integration of the turbulent-molecular transport equation (with a chemical source term) in the ocean. It extends previous work that only considered reactions within the oceanic molecular sublayer. The sensitivity of the ocean-side transport to reaction rate and wind forcing is examined. A more complicated case with a much more reactive thin surfactant layer is also considered. The full atmosphere-ocean deposition velocity is obtained by matching boundary conditions at the interface. For an assumed ocean reaction rate of 103 s¿1, the enhancement for ozone deposition by oceanic turbulence is found to be up to a factor of three for meteorological data obtained in a recent cruise off the East Coast of the U.S. en application/pdf https://research.wur.nl/en/publications/water-side-turbulence-enhancement-of-ozone-deposition-to-the-ocea https://edepot.wur.nl/10281 boundary-layer dry deposition fluxes gas-exchange parameterization surface trends wind-speed Wageningen University & Research
institution WUR NL
collection DSpace
country Países bajos
countrycode NL
component Bibliográfico
access En linea
databasecode dig-wur-nl
tag biblioteca
region Europa del Oeste
libraryname WUR Library Netherlands
language English
topic boundary-layer
dry deposition
fluxes
gas-exchange
parameterization
surface
trends
wind-speed
boundary-layer
dry deposition
fluxes
gas-exchange
parameterization
surface
trends
wind-speed
spellingShingle boundary-layer
dry deposition
fluxes
gas-exchange
parameterization
surface
trends
wind-speed
boundary-layer
dry deposition
fluxes
gas-exchange
parameterization
surface
trends
wind-speed
Fairall, C.W.
Helmig, D.
Ganzeveld, L.N.
Hare, J.
Water-side turbulence enhancement of ozone deposition to the ocean
description A parameterization for the deposition velocity of an ocean-reactive atmospheric gas (such as ozone) is developed. The parameterization is based on integration of the turbulent-molecular transport equation (with a chemical source term) in the ocean. It extends previous work that only considered reactions within the oceanic molecular sublayer. The sensitivity of the ocean-side transport to reaction rate and wind forcing is examined. A more complicated case with a much more reactive thin surfactant layer is also considered. The full atmosphere-ocean deposition velocity is obtained by matching boundary conditions at the interface. For an assumed ocean reaction rate of 103 s¿1, the enhancement for ozone deposition by oceanic turbulence is found to be up to a factor of three for meteorological data obtained in a recent cruise off the East Coast of the U.S.
format Article/Letter to editor
topic_facet boundary-layer
dry deposition
fluxes
gas-exchange
parameterization
surface
trends
wind-speed
author Fairall, C.W.
Helmig, D.
Ganzeveld, L.N.
Hare, J.
author_facet Fairall, C.W.
Helmig, D.
Ganzeveld, L.N.
Hare, J.
author_sort Fairall, C.W.
title Water-side turbulence enhancement of ozone deposition to the ocean
title_short Water-side turbulence enhancement of ozone deposition to the ocean
title_full Water-side turbulence enhancement of ozone deposition to the ocean
title_fullStr Water-side turbulence enhancement of ozone deposition to the ocean
title_full_unstemmed Water-side turbulence enhancement of ozone deposition to the ocean
title_sort water-side turbulence enhancement of ozone deposition to the ocean
url https://research.wur.nl/en/publications/water-side-turbulence-enhancement-of-ozone-deposition-to-the-ocea
work_keys_str_mv AT fairallcw watersideturbulenceenhancementofozonedepositiontotheocean
AT helmigd watersideturbulenceenhancementofozonedepositiontotheocean
AT ganzeveldln watersideturbulenceenhancementofozonedepositiontotheocean
AT harej watersideturbulenceenhancementofozonedepositiontotheocean
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