Reconciliation of essential process parameters for an enhanced predictability of Arctic stratospheric ozone loss and its climate interactions (RECONCILE) : Activities and results

The international research project RECONCILE has addressed central questions regarding polar ozone depletion, with the objective to quantify some of the most relevant yet still uncertain physical and chemical processes and thereby improve prognostic modelling capabilities to realistically predict the response of the ozone layer to climate change. This overview paper outlines the scope and the general approach of RECONCILE, and it provides a summary of observations and modelling in 2010 and 2011 that have generated an in many respects unprecedented dataset to study processes in the Arctic winter stratosphere. Principally, it summarises important outcomes of RECONCILE including (i) better constraints and enhanced consistency on the set of parameters governing catalytic ozone destruction cycles, (ii) a better understanding of the role of cold binary aerosols in heterogeneous chlorine activation, (iii) an improved scheme of polar stratospheric cloud (PSC) processes that includes heterogeneous nucleation of nitric acid trihydrate (NAT) and ice on non-volatile background aerosol leading to better model parameterisations with respect to denitrification, and (iv) long transient simulations with a chemistry-climate model (CCM) updated based on the results of RECONCILE that better reproduce past ozone trends in Antarctica and are deemed to produce more reliable predictions of future ozone trends. The process studies and the global simulations conducted in RECONCILE show that in the Arctic, ozone depletion uncertainties in the chemical and microphysical processes are now clearly smaller than the sensitivity to dynamic variability.

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Main Authors: Von Hobe, M., Bekki, S., Borrmann, S., Cairo, F., D'Amato, F., Di Donfrancesco, G., Dörnbrack, A., Ebersoldt, A., Ebert, M., Emde, C., Engel, I., Ern, M., Frey, W., Genco, S., Griessbach, S., Grooß, J.U., Gulde, T., Günther, G., Hösen, E., Hoffmann, L., Homonnai, V., Hoyle, C.R., Isaksen, I.S.A., Jackson, D.R., Jánosi, I.M., Jones, R.L., Kandler, K., Kalicinsky, C., Keil, A., Khaykin, S.M., Khosrawi, F., Kivi, R., Kuttippurath, J., Laube, J.C., Lefèvre, F., Lehmann, R., Ludmann, S., Luo, B.P., Marchand, M., Meyer, J., Mitev, V., Molleker, S., Müller, R., Oelhaf, H., Olschewski, F., Orsolini, Y., Peter, T., Pfeilsticker, K., Piesch, C., Pitts, M.C., Poole, L.R., Pope, F.D., Ravegnani, F., Rex, M., Riese, M., Röckmann, T., Rognerud, B., Roiger, A., Rolf, C., Santee, M.L., Scheibe, M., Schiller, C., Schlager, H., Siciliani De Cumis, M., Sitnikov, N., Søvde, O.A., Spang, R., Spelten, N., Stordal, F., Sumiñska-Ebersoldt, O., Ulanovski, A., Ungermann, J., Viciani, S., Volk, C.M., Vom Scheidt, M., Von Der Gathen, P., Walker, K., Wegner, T., Weigel, R., Weinbruch, S., Wetzel, G., Wienhold, F.G., Wohltmann, I., Woiwode, W., Young, I.A.K., Yushkov, V., Zobrist, B., Stroh, F.
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Subjects:Life Science,
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spelling dig-wur-nl-wurpubs-6142842024-05-14 Von Hobe, M. Bekki, S. Borrmann, S. Cairo, F. D'Amato, F. Di Donfrancesco, G. Dörnbrack, A. Ebersoldt, A. Ebert, M. Emde, C. Engel, I. Ern, M. Frey, W. Genco, S. Griessbach, S. Grooß, J.U. Gulde, T. Günther, G. Hösen, E. Hoffmann, L. Homonnai, V. Hoyle, C.R. Isaksen, I.S.A. Jackson, D.R. Jánosi, I.M. Jones, R.L. Kandler, K. Kalicinsky, C. Keil, A. Khaykin, S.M. Khosrawi, F. Kivi, R. Kuttippurath, J. Laube, J.C. Lefèvre, F. Lehmann, R. Ludmann, S. Luo, B.P. Marchand, M. Meyer, J. Mitev, V. Molleker, S. Müller, R. Oelhaf, H. Olschewski, F. Orsolini, Y. Peter, T. Pfeilsticker, K. Piesch, C. Pitts, M.C. Poole, L.R. Pope, F.D. Ravegnani, F. Rex, M. Riese, M. Röckmann, T. Rognerud, B. Roiger, A. Rolf, C. Santee, M.L. Scheibe, M. Schiller, C. Schlager, H. Siciliani De Cumis, M. Sitnikov, N. Søvde, O.A. Spang, R. Spelten, N. Stordal, F. Sumiñska-Ebersoldt, O. Ulanovski, A. Ungermann, J. Viciani, S. Volk, C.M. Vom Scheidt, M. Von Der Gathen, P. Walker, K. Wegner, T. Weigel, R. Weinbruch, S. Wetzel, G. Wienhold, F.G. Wohltmann, I. Woiwode, W. Young, I.A.K. Yushkov, V. Zobrist, B. Stroh, F. Article/Letter to editor Atmospheric Chemistry and Physics 13 (2013) 18 ISSN: 1680-7316 Reconciliation of essential process parameters for an enhanced predictability of Arctic stratospheric ozone loss and its climate interactions (RECONCILE) : Activities and results 2013 The international research project RECONCILE has addressed central questions regarding polar ozone depletion, with the objective to quantify some of the most relevant yet still uncertain physical and chemical processes and thereby improve prognostic modelling capabilities to realistically predict the response of the ozone layer to climate change. This overview paper outlines the scope and the general approach of RECONCILE, and it provides a summary of observations and modelling in 2010 and 2011 that have generated an in many respects unprecedented dataset to study processes in the Arctic winter stratosphere. Principally, it summarises important outcomes of RECONCILE including (i) better constraints and enhanced consistency on the set of parameters governing catalytic ozone destruction cycles, (ii) a better understanding of the role of cold binary aerosols in heterogeneous chlorine activation, (iii) an improved scheme of polar stratospheric cloud (PSC) processes that includes heterogeneous nucleation of nitric acid trihydrate (NAT) and ice on non-volatile background aerosol leading to better model parameterisations with respect to denitrification, and (iv) long transient simulations with a chemistry-climate model (CCM) updated based on the results of RECONCILE that better reproduce past ozone trends in Antarctica and are deemed to produce more reliable predictions of future ozone trends. The process studies and the global simulations conducted in RECONCILE show that in the Arctic, ozone depletion uncertainties in the chemical and microphysical processes are now clearly smaller than the sensitivity to dynamic variability. en text/html https://research.wur.nl/en/publications/reconciliation-of-essential-process-parameters-for-an-enhanced-pr 10.5194/acp-13-9233-2013 https://edepot.wur.nl/630291 Life Science https://creativecommons.org/licenses/by/4.0/ Wageningen University & Research
institution WUR NL
collection DSpace
country Países bajos
countrycode NL
component Bibliográfico
access En linea
databasecode dig-wur-nl
tag biblioteca
region Europa del Oeste
libraryname WUR Library Netherlands
language English
topic Life Science
Life Science
spellingShingle Life Science
Life Science
Von Hobe, M.
Bekki, S.
Borrmann, S.
Cairo, F.
D'Amato, F.
Di Donfrancesco, G.
Dörnbrack, A.
Ebersoldt, A.
Ebert, M.
Emde, C.
Engel, I.
Ern, M.
Frey, W.
Genco, S.
Griessbach, S.
Grooß, J.U.
Gulde, T.
Günther, G.
Hösen, E.
Hoffmann, L.
Homonnai, V.
Hoyle, C.R.
Isaksen, I.S.A.
Jackson, D.R.
Jánosi, I.M.
Jones, R.L.
Kandler, K.
Kalicinsky, C.
Keil, A.
Khaykin, S.M.
Khosrawi, F.
Kivi, R.
Kuttippurath, J.
Laube, J.C.
Lefèvre, F.
Lehmann, R.
Ludmann, S.
Luo, B.P.
Marchand, M.
Meyer, J.
Mitev, V.
Molleker, S.
Müller, R.
Oelhaf, H.
Olschewski, F.
Orsolini, Y.
Peter, T.
Pfeilsticker, K.
Piesch, C.
Pitts, M.C.
Poole, L.R.
Pope, F.D.
Ravegnani, F.
Rex, M.
Riese, M.
Röckmann, T.
Rognerud, B.
Roiger, A.
Rolf, C.
Santee, M.L.
Scheibe, M.
Schiller, C.
Schlager, H.
Siciliani De Cumis, M.
Sitnikov, N.
Søvde, O.A.
Spang, R.
Spelten, N.
Stordal, F.
Sumiñska-Ebersoldt, O.
Ulanovski, A.
Ungermann, J.
Viciani, S.
Volk, C.M.
Vom Scheidt, M.
Von Der Gathen, P.
Walker, K.
Wegner, T.
Weigel, R.
Weinbruch, S.
Wetzel, G.
Wienhold, F.G.
Wohltmann, I.
Woiwode, W.
Young, I.A.K.
Yushkov, V.
Zobrist, B.
Stroh, F.
Reconciliation of essential process parameters for an enhanced predictability of Arctic stratospheric ozone loss and its climate interactions (RECONCILE) : Activities and results
description The international research project RECONCILE has addressed central questions regarding polar ozone depletion, with the objective to quantify some of the most relevant yet still uncertain physical and chemical processes and thereby improve prognostic modelling capabilities to realistically predict the response of the ozone layer to climate change. This overview paper outlines the scope and the general approach of RECONCILE, and it provides a summary of observations and modelling in 2010 and 2011 that have generated an in many respects unprecedented dataset to study processes in the Arctic winter stratosphere. Principally, it summarises important outcomes of RECONCILE including (i) better constraints and enhanced consistency on the set of parameters governing catalytic ozone destruction cycles, (ii) a better understanding of the role of cold binary aerosols in heterogeneous chlorine activation, (iii) an improved scheme of polar stratospheric cloud (PSC) processes that includes heterogeneous nucleation of nitric acid trihydrate (NAT) and ice on non-volatile background aerosol leading to better model parameterisations with respect to denitrification, and (iv) long transient simulations with a chemistry-climate model (CCM) updated based on the results of RECONCILE that better reproduce past ozone trends in Antarctica and are deemed to produce more reliable predictions of future ozone trends. The process studies and the global simulations conducted in RECONCILE show that in the Arctic, ozone depletion uncertainties in the chemical and microphysical processes are now clearly smaller than the sensitivity to dynamic variability.
format Article/Letter to editor
topic_facet Life Science
author Von Hobe, M.
Bekki, S.
Borrmann, S.
Cairo, F.
D'Amato, F.
Di Donfrancesco, G.
Dörnbrack, A.
Ebersoldt, A.
Ebert, M.
Emde, C.
Engel, I.
Ern, M.
Frey, W.
Genco, S.
Griessbach, S.
Grooß, J.U.
Gulde, T.
Günther, G.
Hösen, E.
Hoffmann, L.
Homonnai, V.
Hoyle, C.R.
Isaksen, I.S.A.
Jackson, D.R.
Jánosi, I.M.
Jones, R.L.
Kandler, K.
Kalicinsky, C.
Keil, A.
Khaykin, S.M.
Khosrawi, F.
Kivi, R.
Kuttippurath, J.
Laube, J.C.
Lefèvre, F.
Lehmann, R.
Ludmann, S.
Luo, B.P.
Marchand, M.
Meyer, J.
Mitev, V.
Molleker, S.
Müller, R.
Oelhaf, H.
Olschewski, F.
Orsolini, Y.
Peter, T.
Pfeilsticker, K.
Piesch, C.
Pitts, M.C.
Poole, L.R.
Pope, F.D.
Ravegnani, F.
Rex, M.
Riese, M.
Röckmann, T.
Rognerud, B.
Roiger, A.
Rolf, C.
Santee, M.L.
Scheibe, M.
Schiller, C.
Schlager, H.
Siciliani De Cumis, M.
Sitnikov, N.
Søvde, O.A.
Spang, R.
Spelten, N.
Stordal, F.
Sumiñska-Ebersoldt, O.
Ulanovski, A.
Ungermann, J.
Viciani, S.
Volk, C.M.
Vom Scheidt, M.
Von Der Gathen, P.
Walker, K.
Wegner, T.
Weigel, R.
Weinbruch, S.
Wetzel, G.
Wienhold, F.G.
Wohltmann, I.
Woiwode, W.
Young, I.A.K.
Yushkov, V.
Zobrist, B.
Stroh, F.
author_facet Von Hobe, M.
Bekki, S.
Borrmann, S.
Cairo, F.
D'Amato, F.
Di Donfrancesco, G.
Dörnbrack, A.
Ebersoldt, A.
Ebert, M.
Emde, C.
Engel, I.
Ern, M.
Frey, W.
Genco, S.
Griessbach, S.
Grooß, J.U.
Gulde, T.
Günther, G.
Hösen, E.
Hoffmann, L.
Homonnai, V.
Hoyle, C.R.
Isaksen, I.S.A.
Jackson, D.R.
Jánosi, I.M.
Jones, R.L.
Kandler, K.
Kalicinsky, C.
Keil, A.
Khaykin, S.M.
Khosrawi, F.
Kivi, R.
Kuttippurath, J.
Laube, J.C.
Lefèvre, F.
Lehmann, R.
Ludmann, S.
Luo, B.P.
Marchand, M.
Meyer, J.
Mitev, V.
Molleker, S.
Müller, R.
Oelhaf, H.
Olschewski, F.
Orsolini, Y.
Peter, T.
Pfeilsticker, K.
Piesch, C.
Pitts, M.C.
Poole, L.R.
Pope, F.D.
Ravegnani, F.
Rex, M.
Riese, M.
Röckmann, T.
Rognerud, B.
Roiger, A.
Rolf, C.
Santee, M.L.
Scheibe, M.
Schiller, C.
Schlager, H.
Siciliani De Cumis, M.
Sitnikov, N.
Søvde, O.A.
Spang, R.
Spelten, N.
Stordal, F.
Sumiñska-Ebersoldt, O.
Ulanovski, A.
Ungermann, J.
Viciani, S.
Volk, C.M.
Vom Scheidt, M.
Von Der Gathen, P.
Walker, K.
Wegner, T.
Weigel, R.
Weinbruch, S.
Wetzel, G.
Wienhold, F.G.
Wohltmann, I.
Woiwode, W.
Young, I.A.K.
Yushkov, V.
Zobrist, B.
Stroh, F.
author_sort Von Hobe, M.
title Reconciliation of essential process parameters for an enhanced predictability of Arctic stratospheric ozone loss and its climate interactions (RECONCILE) : Activities and results
title_short Reconciliation of essential process parameters for an enhanced predictability of Arctic stratospheric ozone loss and its climate interactions (RECONCILE) : Activities and results
title_full Reconciliation of essential process parameters for an enhanced predictability of Arctic stratospheric ozone loss and its climate interactions (RECONCILE) : Activities and results
title_fullStr Reconciliation of essential process parameters for an enhanced predictability of Arctic stratospheric ozone loss and its climate interactions (RECONCILE) : Activities and results
title_full_unstemmed Reconciliation of essential process parameters for an enhanced predictability of Arctic stratospheric ozone loss and its climate interactions (RECONCILE) : Activities and results
title_sort reconciliation of essential process parameters for an enhanced predictability of arctic stratospheric ozone loss and its climate interactions (reconcile) : activities and results
url https://research.wur.nl/en/publications/reconciliation-of-essential-process-parameters-for-an-enhanced-pr
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AT wegnert reconciliationofessentialprocessparametersforanenhancedpredictabilityofarcticstratosphericozonelossanditsclimateinteractionsreconcileactivitiesandresults
AT weigelr reconciliationofessentialprocessparametersforanenhancedpredictabilityofarcticstratosphericozonelossanditsclimateinteractionsreconcileactivitiesandresults
AT weinbruchs reconciliationofessentialprocessparametersforanenhancedpredictabilityofarcticstratosphericozonelossanditsclimateinteractionsreconcileactivitiesandresults
AT wetzelg reconciliationofessentialprocessparametersforanenhancedpredictabilityofarcticstratosphericozonelossanditsclimateinteractionsreconcileactivitiesandresults
AT wienholdfg reconciliationofessentialprocessparametersforanenhancedpredictabilityofarcticstratosphericozonelossanditsclimateinteractionsreconcileactivitiesandresults
AT wohltmanni reconciliationofessentialprocessparametersforanenhancedpredictabilityofarcticstratosphericozonelossanditsclimateinteractionsreconcileactivitiesandresults
AT woiwodew reconciliationofessentialprocessparametersforanenhancedpredictabilityofarcticstratosphericozonelossanditsclimateinteractionsreconcileactivitiesandresults
AT youngiak reconciliationofessentialprocessparametersforanenhancedpredictabilityofarcticstratosphericozonelossanditsclimateinteractionsreconcileactivitiesandresults
AT yushkovv reconciliationofessentialprocessparametersforanenhancedpredictabilityofarcticstratosphericozonelossanditsclimateinteractionsreconcileactivitiesandresults
AT zobristb reconciliationofessentialprocessparametersforanenhancedpredictabilityofarcticstratosphericozonelossanditsclimateinteractionsreconcileactivitiesandresults
AT strohf reconciliationofessentialprocessparametersforanenhancedpredictabilityofarcticstratosphericozonelossanditsclimateinteractionsreconcileactivitiesandresults
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