Soil as an archive of coal-fired power plant mercury deposition
Mercury pollution is a global environmental problem that has serious implications for human health. One of the most important sources of anthropogenic mercury emissions are coal-burning power plants. Hg accumulations in soil are associated with their atmospheric deposition. Our study provides the first assessment of soil Hg on the entire Spanish surface obtained from one sampling protocol. Hg spatial distribution was analysed with topsoil samples taken from 4000 locations in a regular sampling grid. The other aim was to use geostatistical techniques to verify the extent of soil contamination by Hg and to evaluate presumed Hg enrichment near the seven Spanish power plants with installed capacity above 1000MW. The Hg concentration in Spanish soil fell within the range of 1-7564μgkg-1 (mean 67.2) and 50% of the samples had a concentration below 37μgkg-1. Evidence for human activity was found near all the coal-fired power plants, which reflects that metals have accumulated in the basin over many years. Values over 1000μgkg-1 have been found in soils in the vicinity of the Aboño, Soto de Ribera and Castellon power plants. However, soil Hg enrichment was detectable only close to the emission source, within an approximate range of only 15km from the power plants. We associated this effect with airborne emissions and subsequent depositions as the potential distance through fly ash deposition. Hg associated with particles of ash tends to be deposited near coal combustion sources. © 2016 Elsevier B.V.
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Format: | artículo biblioteca |
Language: | English |
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Elsevier
2016
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Subjects: | Heavy metal, Soil mercury-enriched, Coal-fired power plant, Mercury deposition, Geostatistic, |
Online Access: | http://hdl.handle.net/20.500.12792/3804 http://hdl.handle.net/10261/291914 |
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dig-inia-es-10261-2919142023-02-20T07:23:35Z Soil as an archive of coal-fired power plant mercury deposition Rodríguez Martín, José Antonio Nanos, N. Heavy metal Soil mercury-enriched Coal-fired power plant Mercury deposition Geostatistic Mercury pollution is a global environmental problem that has serious implications for human health. One of the most important sources of anthropogenic mercury emissions are coal-burning power plants. Hg accumulations in soil are associated with their atmospheric deposition. Our study provides the first assessment of soil Hg on the entire Spanish surface obtained from one sampling protocol. Hg spatial distribution was analysed with topsoil samples taken from 4000 locations in a regular sampling grid. The other aim was to use geostatistical techniques to verify the extent of soil contamination by Hg and to evaluate presumed Hg enrichment near the seven Spanish power plants with installed capacity above 1000MW. The Hg concentration in Spanish soil fell within the range of 1-7564μgkg-1 (mean 67.2) and 50% of the samples had a concentration below 37μgkg-1. Evidence for human activity was found near all the coal-fired power plants, which reflects that metals have accumulated in the basin over many years. Values over 1000μgkg-1 have been found in soils in the vicinity of the Aboño, Soto de Ribera and Castellon power plants. However, soil Hg enrichment was detectable only close to the emission source, within an approximate range of only 15km from the power plants. We associated this effect with airborne emissions and subsequent depositions as the potential distance through fly ash deposition. Hg associated with particles of ash tends to be deposited near coal combustion sources. © 2016 Elsevier B.V. 2023-02-20T07:23:35Z 2023-02-20T07:23:35Z 2016 artículo Journal of Hazardous Materials 308: 131-138 (2016) 0304-3894 http://hdl.handle.net/20.500.12792/3804 http://hdl.handle.net/10261/291914 10.1016/j.jhazmat.2016.01.026 en none Elsevier |
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Heavy metal Soil mercury-enriched Coal-fired power plant Mercury deposition Geostatistic Heavy metal Soil mercury-enriched Coal-fired power plant Mercury deposition Geostatistic |
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Heavy metal Soil mercury-enriched Coal-fired power plant Mercury deposition Geostatistic Heavy metal Soil mercury-enriched Coal-fired power plant Mercury deposition Geostatistic Rodríguez Martín, José Antonio Nanos, N. Soil as an archive of coal-fired power plant mercury deposition |
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Mercury pollution is a global environmental problem that has serious implications for human health. One of the most important sources of anthropogenic mercury emissions are coal-burning power plants. Hg accumulations in soil are associated with their atmospheric deposition. Our study provides the first assessment of soil Hg on the entire Spanish surface obtained from one sampling protocol. Hg spatial distribution was analysed with topsoil samples taken from 4000 locations in a regular sampling grid. The other aim was to use geostatistical techniques to verify the extent of soil contamination by Hg and to evaluate presumed Hg enrichment near the seven Spanish power plants with installed capacity above 1000MW. The Hg concentration in Spanish soil fell within the range of 1-7564μgkg-1 (mean 67.2) and 50% of the samples had a concentration below 37μgkg-1. Evidence for human activity was found near all the coal-fired power plants, which reflects that metals have accumulated in the basin over many years. Values over 1000μgkg-1 have been found in soils in the vicinity of the Aboño, Soto de Ribera and Castellon power plants. However, soil Hg enrichment was detectable only close to the emission source, within an approximate range of only 15km from the power plants. We associated this effect with airborne emissions and subsequent depositions as the potential distance through fly ash deposition. Hg associated with particles of ash tends to be deposited near coal combustion sources. © 2016 Elsevier B.V. |
format |
artículo |
topic_facet |
Heavy metal Soil mercury-enriched Coal-fired power plant Mercury deposition Geostatistic |
author |
Rodríguez Martín, José Antonio Nanos, N. |
author_facet |
Rodríguez Martín, José Antonio Nanos, N. |
author_sort |
Rodríguez Martín, José Antonio |
title |
Soil as an archive of coal-fired power plant mercury deposition |
title_short |
Soil as an archive of coal-fired power plant mercury deposition |
title_full |
Soil as an archive of coal-fired power plant mercury deposition |
title_fullStr |
Soil as an archive of coal-fired power plant mercury deposition |
title_full_unstemmed |
Soil as an archive of coal-fired power plant mercury deposition |
title_sort |
soil as an archive of coal-fired power plant mercury deposition |
publisher |
Elsevier |
publishDate |
2016 |
url |
http://hdl.handle.net/20.500.12792/3804 http://hdl.handle.net/10261/291914 |
work_keys_str_mv |
AT rodriguezmartinjoseantonio soilasanarchiveofcoalfiredpowerplantmercurydeposition AT nanosn soilasanarchiveofcoalfiredpowerplantmercurydeposition |
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1767603272621752320 |