Outdoor infiltration and indoor contribution of UFP and BC, OC, secondary inorganic ions and metals in PM2.5 in schools

© 2015 The Authors. Infiltration of outdoor-sourced particles into indoor environments in 39 schools in Barcelona was assessed during school hours. Tracers of road traffic emissions (NO2, Equivalent Black Carbon (EBC), Ultrafine Particles (UFP), Sb), secondary inorganic aerosols (SO4 2-, NO3 -, NH4 +) and a number of PM2.5 trace elements showed median indoor/outdoor (I/O) ratios≤1, indicating that outdoor sources importantly contributed to indoor concentrations. Conversely, OC and mineral components had I/O ratios>1. Different infiltration factors were found for traffic and secondary components (0.31-0.75 and 0.50-0.92, cold and warm season respectively), with maxima corresponding to EBC and Cd. Higher concentrations of indoor-generated particles were observed when closed windows hindered dispersion (cold season). Building age was not a major determinant of indoor levels. Neither were the window's material, except for NO2 (with an increase of 8μgm-3 for wood framed windows) and the mineral components (also dependent on the presence of sand in a distance <20m) that reach the indoor environment via soil adhering to footwear with their dispersion being more barred by Aluminium/PVC framed windows than the wooden ones. Enlarged indoor concentrations of some trace elements suggest the presence of indoor sources that should be further investigated in order to achieve a healthier school indoor environment.

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Main Authors: Rivas, Ioar, Viana, Mar, Moreno, Teresa, Bouso, L., Pandolfi, Marco, Álvarez-Pedrerol, Mar, Forns, Joan, Alastuey, Andrés, Sunyer, J., Querol, Xavier
Other Authors: European Commission
Format: artículo biblioteca
Published: 2015
Online Access:http://hdl.handle.net/10261/218793
http://dx.doi.org/10.13039/501100000780
http://dx.doi.org/10.13039/501100002809
http://dx.doi.org/10.13039/501100004837
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spelling dig-idaea-es-10261-2187932022-06-14T07:28:12Z Outdoor infiltration and indoor contribution of UFP and BC, OC, secondary inorganic ions and metals in PM2.5 in schools Rivas, Ioar Viana, Mar Moreno, Teresa Bouso, L. Pandolfi, Marco Álvarez-Pedrerol, Mar Forns, Joan Alastuey, Andrés Sunyer, J. Querol, Xavier European Commission Ministerio de Ciencia e Innovación (España) Generalitat de Catalunya © 2015 The Authors. Infiltration of outdoor-sourced particles into indoor environments in 39 schools in Barcelona was assessed during school hours. Tracers of road traffic emissions (NO2, Equivalent Black Carbon (EBC), Ultrafine Particles (UFP), Sb), secondary inorganic aerosols (SO4 2-, NO3 -, NH4 +) and a number of PM2.5 trace elements showed median indoor/outdoor (I/O) ratios≤1, indicating that outdoor sources importantly contributed to indoor concentrations. Conversely, OC and mineral components had I/O ratios>1. Different infiltration factors were found for traffic and secondary components (0.31-0.75 and 0.50-0.92, cold and warm season respectively), with maxima corresponding to EBC and Cd. Higher concentrations of indoor-generated particles were observed when closed windows hindered dispersion (cold season). Building age was not a major determinant of indoor levels. Neither were the window's material, except for NO2 (with an increase of 8μgm-3 for wood framed windows) and the mineral components (also dependent on the presence of sand in a distance <20m) that reach the indoor environment via soil adhering to footwear with their dispersion being more barred by Aluminium/PVC framed windows than the wooden ones. Enlarged indoor concentrations of some trace elements suggest the presence of indoor sources that should be further investigated in order to achieve a healthier school indoor environment. The research leading to these results has received funding from the European Community's Seventh Framework Program (ERC-Advanced Grant) under grant agreement number 268479 – the BREATHE project. Thanks are due to all the participant schools and colleagues. Additional instrumentation was kindly provided by national projects IMPACT (CGL2011-26574), VAMOS (CLG2010-19464-CLI) and CECAT (CTM2011-14730-E). Support from the Generalitat de Catalunya 2015 SGR33is gratefully acknowledged. 2020-08-28T08:00:47Z 2020-08-28T08:00:47Z 2015 2020-08-28T08:00:48Z artículo http://purl.org/coar/resource_type/c_6501 doi: 10.1016/j.atmosenv.2015.01.055 issn: 1873-2844 Atmospheric Environment 106: 129-138 (2015) http://hdl.handle.net/10261/218793 10.1016/j.atmosenv.2015.01.055 http://dx.doi.org/10.13039/501100000780 http://dx.doi.org/10.13039/501100002809 http://dx.doi.org/10.13039/501100004837 #PLACEHOLDER_PARENT_METADATA_VALUE# info:eu-repo/grantAgreement/EC/FP7/268479 Publisher's version http://dx.doi.org/10.1016/j.atmosenv.2015.01.055 Sí open
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libraryname Biblioteca del IDAEA España
description © 2015 The Authors. Infiltration of outdoor-sourced particles into indoor environments in 39 schools in Barcelona was assessed during school hours. Tracers of road traffic emissions (NO2, Equivalent Black Carbon (EBC), Ultrafine Particles (UFP), Sb), secondary inorganic aerosols (SO4 2-, NO3 -, NH4 +) and a number of PM2.5 trace elements showed median indoor/outdoor (I/O) ratios≤1, indicating that outdoor sources importantly contributed to indoor concentrations. Conversely, OC and mineral components had I/O ratios>1. Different infiltration factors were found for traffic and secondary components (0.31-0.75 and 0.50-0.92, cold and warm season respectively), with maxima corresponding to EBC and Cd. Higher concentrations of indoor-generated particles were observed when closed windows hindered dispersion (cold season). Building age was not a major determinant of indoor levels. Neither were the window's material, except for NO2 (with an increase of 8μgm-3 for wood framed windows) and the mineral components (also dependent on the presence of sand in a distance <20m) that reach the indoor environment via soil adhering to footwear with their dispersion being more barred by Aluminium/PVC framed windows than the wooden ones. Enlarged indoor concentrations of some trace elements suggest the presence of indoor sources that should be further investigated in order to achieve a healthier school indoor environment.
author2 European Commission
author_facet European Commission
Rivas, Ioar
Viana, Mar
Moreno, Teresa
Bouso, L.
Pandolfi, Marco
Álvarez-Pedrerol, Mar
Forns, Joan
Alastuey, Andrés
Sunyer, J.
Querol, Xavier
format artículo
author Rivas, Ioar
Viana, Mar
Moreno, Teresa
Bouso, L.
Pandolfi, Marco
Álvarez-Pedrerol, Mar
Forns, Joan
Alastuey, Andrés
Sunyer, J.
Querol, Xavier
spellingShingle Rivas, Ioar
Viana, Mar
Moreno, Teresa
Bouso, L.
Pandolfi, Marco
Álvarez-Pedrerol, Mar
Forns, Joan
Alastuey, Andrés
Sunyer, J.
Querol, Xavier
Outdoor infiltration and indoor contribution of UFP and BC, OC, secondary inorganic ions and metals in PM2.5 in schools
author_sort Rivas, Ioar
title Outdoor infiltration and indoor contribution of UFP and BC, OC, secondary inorganic ions and metals in PM2.5 in schools
title_short Outdoor infiltration and indoor contribution of UFP and BC, OC, secondary inorganic ions and metals in PM2.5 in schools
title_full Outdoor infiltration and indoor contribution of UFP and BC, OC, secondary inorganic ions and metals in PM2.5 in schools
title_fullStr Outdoor infiltration and indoor contribution of UFP and BC, OC, secondary inorganic ions and metals in PM2.5 in schools
title_full_unstemmed Outdoor infiltration and indoor contribution of UFP and BC, OC, secondary inorganic ions and metals in PM2.5 in schools
title_sort outdoor infiltration and indoor contribution of ufp and bc, oc, secondary inorganic ions and metals in pm2.5 in schools
publishDate 2015
url http://hdl.handle.net/10261/218793
http://dx.doi.org/10.13039/501100000780
http://dx.doi.org/10.13039/501100002809
http://dx.doi.org/10.13039/501100004837
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