Waste biomass valorisation for the development of sustainable cellulosic aerogels and their sound absorption properties
Novel and more sustainable sound absorbing materials are produced through the valorization of waste biomass sources by following circular economy principles. Cellulosic nanocrystals (CNC) were extracted from Posidonia oceanica dead leaves, spent barely grains, and kale stems (KS) using a simplified purification protocol. These nanocrystals are used to prepare cellulosic aerogels, evaluating the effect of three parameters, namely, concentration (0.5–4%), CaCl2 and poly(lactic acid) (PLA) incorporation (hybrid aerogels), on their sound absorption properties. Aerogels from 4% suspensions show the highest sound absorption, outperforming benchmark rockwool and polyester—two modern commonly-used sound absorbers. Moreover, PLA coating also improves the sound absorption performance of the most aerogels. CNC from KS aerogels are selected as the optimum at both high (500–6000 Hz) and low (100–1500 Hz) frequency ranges. Overall, these results represent a new proof-of-concept of waste biomass conversion to high-performance cellulosic aerogels that have excellent sound absorbing properties.
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Format: | artículo biblioteca |
Language: | English |
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John Wiley & Sons
2022-08-30
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Subjects: | Aerogels, Biomass valorisation, Cellulosic nanocrystals, Poly(lactic acid), Sound absorption, |
Online Access: | http://hdl.handle.net/10261/281944 http://dx.doi.org/10.13039/501100002341 http://dx.doi.org/10.13039/501100000780 http://dx.doi.org/10.13039/501100004837 http://dx.doi.org/10.13039/501100003339 http://dx.doi.org/10.13039/501100011033 https://api.elsevier.com/content/abstract/scopus_id/85137024532 |
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dig-iata-es-10261-2819442024-10-27T22:23:14Z Waste biomass valorisation for the development of sustainable cellulosic aerogels and their sound absorption properties Benito González, Isaac Cucharero, Jose Al Haj, Yazan Hänninen, Tuomas Lokki, Tapio Martínez Sanz, Marta López-Rubio, Amparo Martínez-Abad, Antonio Vapaavuori, Jaana European Commission Ministerio de Ciencia e Innovación (España) Academy of Finland Consejo Superior de Investigaciones Científicas (España) Ministerio de Ciencia, Innovación y Universidades (España) Agencia Estatal de Investigación (España) 0000-0002-5923-0789 Consejo Superior de Investigaciones Científicas [https://ror.org/02gfc7t72] Aerogels Biomass valorisation Cellulosic nanocrystals Poly(lactic acid) Sound absorption Novel and more sustainable sound absorbing materials are produced through the valorization of waste biomass sources by following circular economy principles. Cellulosic nanocrystals (CNC) were extracted from Posidonia oceanica dead leaves, spent barely grains, and kale stems (KS) using a simplified purification protocol. These nanocrystals are used to prepare cellulosic aerogels, evaluating the effect of three parameters, namely, concentration (0.5–4%), CaCl2 and poly(lactic acid) (PLA) incorporation (hybrid aerogels), on their sound absorption properties. Aerogels from 4% suspensions show the highest sound absorption, outperforming benchmark rockwool and polyester—two modern commonly-used sound absorbers. Moreover, PLA coating also improves the sound absorption performance of the most aerogels. CNC from KS aerogels are selected as the optimum at both high (500–6000 Hz) and low (100–1500 Hz) frequency ranges. Overall, these results represent a new proof-of-concept of waste biomass conversion to high-performance cellulosic aerogels that have excellent sound absorbing properties. This research is part of the CSIC program for the Spanish Recovery, Transformation and Resilience Plan funded by the Recovery and Resilience Facility of the European Union, established by the Regulation (EU) 2020/2094. Grant RTI2018-094268-B-C22 funded by MCIN/AEI/ 10.13039/501100011033 and by “ERDF A way of making Europe”. This work was a part of the Academy of Finland's Flagship Programme under Projects No. 318890 and 318891 (Competence Center for Materials Bioeconomy, FinnCERES). Peer reviewed 2022-11-02T07:29:44Z 2022-11-02T07:29:44Z 2022-08-30 artículo http://purl.org/coar/resource_type/c_6501 Advanced Sustainable Systems 6(11): 2200248 (2022) http://hdl.handle.net/10261/281944 10.1002/adsu.202200248 2366-7486 http://dx.doi.org/10.13039/501100002341 http://dx.doi.org/10.13039/501100000780 http://dx.doi.org/10.13039/501100004837 http://dx.doi.org/10.13039/501100003339 http://dx.doi.org/10.13039/501100011033 2-s2.0-85137024532 https://api.elsevier.com/content/abstract/scopus_id/85137024532 en #PLACEHOLDER_PARENT_METADATA_VALUE# info:eu-repo/grantAgreement/AEI/Plan Estatal de Investigación Científica y Técnica y de Innovación 2017-2020/RTI2018-094268-B-C22/ES/MEJORA DE LAS PROPIEDADES TECNOLOGICAS Y NUTRICIONALES DE ALIMENTOS UTILIZANDO GELES Y EMULSIONES FORMADOS A PARTIR DE CARBOHIDRATOS NO PURIFICADOS OBTENIDOS DE FUENTES ALTERN/ Advanced Sustainable Systems Publisher's version The underlying dataset has been published as supplementary material of the article in the publisher platform at DOI 10.1002/adsu.202200248 https://doi.org/10.1002/adsu.202200248 Sí open application/pdf John Wiley & Sons |
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Aerogels Biomass valorisation Cellulosic nanocrystals Poly(lactic acid) Sound absorption Aerogels Biomass valorisation Cellulosic nanocrystals Poly(lactic acid) Sound absorption |
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Aerogels Biomass valorisation Cellulosic nanocrystals Poly(lactic acid) Sound absorption Aerogels Biomass valorisation Cellulosic nanocrystals Poly(lactic acid) Sound absorption Benito González, Isaac Cucharero, Jose Al Haj, Yazan Hänninen, Tuomas Lokki, Tapio Martínez Sanz, Marta López-Rubio, Amparo Martínez-Abad, Antonio Vapaavuori, Jaana Waste biomass valorisation for the development of sustainable cellulosic aerogels and their sound absorption properties |
description |
Novel and more sustainable sound absorbing materials are produced through the valorization of waste biomass sources by following circular economy principles. Cellulosic nanocrystals (CNC) were extracted from Posidonia oceanica dead leaves, spent barely grains, and kale stems (KS) using a simplified purification protocol. These nanocrystals are used to prepare cellulosic aerogels, evaluating the effect of three parameters, namely, concentration (0.5–4%), CaCl2 and poly(lactic acid) (PLA) incorporation (hybrid aerogels), on their sound absorption properties. Aerogels from 4% suspensions show the highest sound absorption, outperforming benchmark rockwool and polyester—two modern commonly-used sound absorbers. Moreover, PLA coating also improves the sound absorption performance of the most aerogels. CNC from KS aerogels are selected as the optimum at both high (500–6000 Hz) and low (100–1500 Hz) frequency ranges. Overall, these results represent a new proof-of-concept of waste biomass conversion to high-performance cellulosic aerogels that have excellent sound absorbing properties. |
author2 |
European Commission |
author_facet |
European Commission Benito González, Isaac Cucharero, Jose Al Haj, Yazan Hänninen, Tuomas Lokki, Tapio Martínez Sanz, Marta López-Rubio, Amparo Martínez-Abad, Antonio Vapaavuori, Jaana |
format |
artículo |
topic_facet |
Aerogels Biomass valorisation Cellulosic nanocrystals Poly(lactic acid) Sound absorption |
author |
Benito González, Isaac Cucharero, Jose Al Haj, Yazan Hänninen, Tuomas Lokki, Tapio Martínez Sanz, Marta López-Rubio, Amparo Martínez-Abad, Antonio Vapaavuori, Jaana |
author_sort |
Benito González, Isaac |
title |
Waste biomass valorisation for the development of sustainable cellulosic aerogels and their sound absorption properties |
title_short |
Waste biomass valorisation for the development of sustainable cellulosic aerogels and their sound absorption properties |
title_full |
Waste biomass valorisation for the development of sustainable cellulosic aerogels and their sound absorption properties |
title_fullStr |
Waste biomass valorisation for the development of sustainable cellulosic aerogels and their sound absorption properties |
title_full_unstemmed |
Waste biomass valorisation for the development of sustainable cellulosic aerogels and their sound absorption properties |
title_sort |
waste biomass valorisation for the development of sustainable cellulosic aerogels and their sound absorption properties |
publisher |
John Wiley & Sons |
publishDate |
2022-08-30 |
url |
http://hdl.handle.net/10261/281944 http://dx.doi.org/10.13039/501100002341 http://dx.doi.org/10.13039/501100000780 http://dx.doi.org/10.13039/501100004837 http://dx.doi.org/10.13039/501100003339 http://dx.doi.org/10.13039/501100011033 https://api.elsevier.com/content/abstract/scopus_id/85137024532 |
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